Study on interface structure and thermal conductivity regulation of Cu–In composite thermal interface materials

Bibliographic Details
Title: Study on interface structure and thermal conductivity regulation of Cu–In composite thermal interface materials
Authors: Jie Zhang, Nan Wu, Hong Guo, Zhongnan Xie, Mingmei Sun, Hui Yang, Ximin Zhang, Yulin Liu, Xinbo He
Source: Journal of Materials Research and Technology, Vol 34, Iss , Pp 1020-1028 (2025)
Publisher Information: Elsevier, 2025.
Publication Year: 2025
Collection: LCC:Mining engineering. Metallurgy
Subject Terms: Thermal interface material, Cu–In composite materials, Hot press sintering, Interface regulation, Thermal conductivity, Mining engineering. Metallurgy, TN1-997
More Details: In foil has excellent heat dissipation performance as a commercially available thermal interface material for high power devices. In order to improve the heat transfer performance of In-based thermal interface materials, a composite thermal interface material with In as the matrix and Cu as the reinforcement was prepared in this research by hot press sintering. The Cu–In composite material's characteristic interfacial structure was examined through the use of transmission electron microscopy. Theoretical models were employed to determine the thermal conduction patterns across various CuIn phase interfaces. By fine-tuning the parameters of the hot press sintering process, we were able to regulate the CuIn phase interface layer's morphology. Results indicate that the Cu–In interface is bonded through a reactive interface, leading to the formation of the CuIn phase that is tightly atomically bonded with both In and Cu. The CuIn phase, when continuous, exhibits higher interfacial thermal conductivity as its thickness decreases. Practical fabrication considerations show that the CuIn phase interface transitions from discontinuous to continuous at a thickness of ∼0.91 μm. Therefore, a continuous CuIn phase interface layer of about 0.91 μm thick yields the highest thermal conductivity, reaching 122.25 Wm−1K−1, which is 1.4 times greater than that of pure In. This research presents innovative choices and strategic directions for advancing the field of high-thermal-conductivity interfacial materials.
Document Type: article
File Description: electronic resource
Language: English
ISSN: 2238-7854
Relation: http://www.sciencedirect.com/science/article/pii/S2238785424029077; https://doaj.org/toc/2238-7854
DOI: 10.1016/j.jmrt.2024.12.104
Access URL: https://doaj.org/article/13fbed25f84a44f3a9e51019dfc81f7b
Accession Number: edsdoj.13fbed25f84a44f3a9e51019dfc81f7b
Database: Directory of Open Access Journals
More Details
ISSN:22387854
DOI:10.1016/j.jmrt.2024.12.104
Published in:Journal of Materials Research and Technology
Language:English