Quantitative Surface Plasmon Interferometry via Upconversion Photoluminescence Mapping

Bibliographic Details
Title: Quantitative Surface Plasmon Interferometry via Upconversion Photoluminescence Mapping
Authors: Anxiang Yin, Hao Jing, Zhan Wu, Qiyuan He, Yiliu Wang, Zhaoyang Lin, Yuan Liu, Mengning Ding, Xu Xu, Zhe Fei, Jianhui Jiang, Yu Huang, Xiangfeng Duan
Source: Research, Vol 2019 (2019)
Publisher Information: American Association for the Advancement of Science (AAAS), 2019.
Publication Year: 2019
Collection: LCC:Science
Subject Terms: Science
More Details: Direct far-field visualization and characterization of surface plasmon polaritons (SPPs) are of great importance for fundamental studies and technological applications. To probe the evanescently confined plasmon fields, one usually requires advanced near-field techniques, which is typically not applicable for real-time, high-throughput detecting or mapping of SPPs in complicated environments. Here, we report the utilization of rare-earth-doped nanoparticles to quantitatively upconvert invisible, evanescently confined SPPs into visible photoluminescence emissions for direct far-field visualization of SPPs in a complicated environment. The observed interference fringes between the SPPs and the coherent incident light at the metal surface provide a quantitative measurement of the SPP wavelength and the SPP propagating length and the local dielectric environments. It thus creates a new signaling pathway to sensitively transduce the local dielectric environment change into interference periodicity variation, enabling a new design of directly measurable, spectrometer-free optical rulers for rapid, ultrasensitive label-free detection of various biomolecules, including streptavidin and prostate-specific antigen, down to the femtomolar level.
Document Type: article
File Description: electronic resource
Language: English
ISSN: 2639-5274
Relation: https://doaj.org/toc/2639-5274
DOI: 10.34133/2019/8304824
Access URL: https://doaj.org/article/0c1280f57bdc49ac8c40de7d0fc26a41
Accession Number: edsdoj.0c1280f57bdc49ac8c40de7d0fc26a41
Database: Directory of Open Access Journals
More Details
ISSN:26395274
DOI:10.34133/2019/8304824
Published in:Research
Language:English