Single photon emitters in thin GaAsN nanowire tubes grown on Si

Bibliographic Details
Title: Single photon emitters in thin GaAsN nanowire tubes grown on Si
Authors: Denis, Nadine, Dede, Didem, Nurmamytov, Timur, Cianci, Salvatore, Santangeli, Francesca, Felici, Marco, Boureau, Victor, Polimeni, Antonio, Rubini, Silvia, Morral, Anna Fontcuberta i, De Luca, Marta
Publication Year: 2024
Collection: Condensed Matter
Physics (Other)
Quantum Physics
Subject Terms: Physics - Optics, Condensed Matter - Materials Science, Quantum Physics
More Details: III-V nanowire heterostructures can act as sources of single and entangled photons and are enabling technologies for on-chip applications in future quantum photonic devices. The unique geometry of nanowires allows to integrate lattice-mismatched components beyond the limits of planar epilayers and to create radially and axially confined quantum structures. Here, we report the plasma-assisted molecular beam epitaxy growth of thin GaAs/GaAsN/GaAs core-multishell nanowires monolithically integrated on Si (111) substrates, overcoming the challenges caused by the low solubility of N and a high lattice mismatch. The nanowires have a GaAsN shell of 10 nm containing 2.7% N, which reduces the GaAs bandgap drastically by 400 meV. They have a symmetric core-shell structure with sharp boundaries and a defect-free zincblende phase. The high structural quality reflects in their excellent opto-electroinic properties, including remarkable single photon emission from quantum confined states in the thin GaAsN shell with a second-order autocorrelation function at zero time delay as low as 0.056.
Document Type: Working Paper
Access URL: http://arxiv.org/abs/2411.03185
Accession Number: edsarx.2411.03185
Database: arXiv
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  Data: Single photon emitters in thin GaAsN nanowire tubes grown on Si
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  Data: <searchLink fieldCode="AR" term="%22Denis%2C+Nadine%22">Denis, Nadine</searchLink><br /><searchLink fieldCode="AR" term="%22Dede%2C+Didem%22">Dede, Didem</searchLink><br /><searchLink fieldCode="AR" term="%22Nurmamytov%2C+Timur%22">Nurmamytov, Timur</searchLink><br /><searchLink fieldCode="AR" term="%22Cianci%2C+Salvatore%22">Cianci, Salvatore</searchLink><br /><searchLink fieldCode="AR" term="%22Santangeli%2C+Francesca%22">Santangeli, Francesca</searchLink><br /><searchLink fieldCode="AR" term="%22Felici%2C+Marco%22">Felici, Marco</searchLink><br /><searchLink fieldCode="AR" term="%22Boureau%2C+Victor%22">Boureau, Victor</searchLink><br /><searchLink fieldCode="AR" term="%22Polimeni%2C+Antonio%22">Polimeni, Antonio</searchLink><br /><searchLink fieldCode="AR" term="%22Rubini%2C+Silvia%22">Rubini, Silvia</searchLink><br /><searchLink fieldCode="AR" term="%22Morral%2C+Anna+Fontcuberta+i%22">Morral, Anna Fontcuberta i</searchLink><br /><searchLink fieldCode="AR" term="%22De+Luca%2C+Marta%22">De Luca, Marta</searchLink>
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  Data: 2024
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  Data: Condensed Matter<br />Physics (Other)<br />Quantum Physics
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  Data: III-V nanowire heterostructures can act as sources of single and entangled photons and are enabling technologies for on-chip applications in future quantum photonic devices. The unique geometry of nanowires allows to integrate lattice-mismatched components beyond the limits of planar epilayers and to create radially and axially confined quantum structures. Here, we report the plasma-assisted molecular beam epitaxy growth of thin GaAs/GaAsN/GaAs core-multishell nanowires monolithically integrated on Si (111) substrates, overcoming the challenges caused by the low solubility of N and a high lattice mismatch. The nanowires have a GaAsN shell of 10 nm containing 2.7% N, which reduces the GaAs bandgap drastically by 400 meV. They have a symmetric core-shell structure with sharp boundaries and a defect-free zincblende phase. The high structural quality reflects in their excellent opto-electroinic properties, including remarkable single photon emission from quantum confined states in the thin GaAsN shell with a second-order autocorrelation function at zero time delay as low as 0.056.
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      – SubjectFull: Physics - Optics
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      – SubjectFull: Condensed Matter - Materials Science
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      – SubjectFull: Quantum Physics
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      – TitleFull: Single photon emitters in thin GaAsN nanowire tubes grown on Si
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              Y: 2024
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