Phase Coexistence and Edge Currents in the Chiral Lennard-Jones Fluid

Bibliographic Details
Title: Phase Coexistence and Edge Currents in the Chiral Lennard-Jones Fluid
Authors: Caporusso, Claudio B., Gonnella, Giuseppe, Levis, Demian
Publication Year: 2023
Collection: Condensed Matter
Subject Terms: Condensed Matter - Soft Condensed Matter, Condensed Matter - Statistical Mechanics
More Details: We study a model chiral fluid in two dimensions composed of Brownian disks interacting via a Lennard-Jones potential and a non-conservative transverse force, mimicking colloids spinning at a rate $\omega$. The system exhibits a phase separation between a chiral liquid and a dilute gas phase that can be characterized using a thermodynamic framework. We compute the equations of state and show that the surface tension controls interface corrections to the coexisting pressure predicted from the equal-area construction. Transverse forces increase surface tension and generate edge currents at the liquid-gas interface. The analysis of these currents shows that the rotational viscosity introduced in chiral hydrodynamics is consistent with microscopic bulk mechanical measurements. Chirality can also break the solid phase, giving rise to a dense fluid made of rotating hexatic patches. Our work paves the way for the development of the statistical mechanics of chiral particles assemblies.
Comment: 6 pages, 4 figures, Supplemental Material
Document Type: Working Paper
Access URL: http://arxiv.org/abs/2307.03528
Accession Number: edsarx.2307.03528
Database: arXiv
More Details
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