Muon spin relaxation and emergence of disorder-induced unconventional dynamic magnetic fluctuations in Dy$_{2}$Zr$_{2}$O$_{7}$

Bibliographic Details
Title: Muon spin relaxation and emergence of disorder-induced unconventional dynamic magnetic fluctuations in Dy$_{2}$Zr$_{2}$O$_{7}$
Authors: Sheetal, Biswas, Pabitra K., Yokoyama, K., Adroja, D. T., Yadav, C. S.
Publication Year: 2023
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science
More Details: The disordered pyrochlore oxide Dy$_{2}$Zr$_{2}$O$_{7}$ shows the signatures of field-induced spin freezing with remnant zero-point spin-ice entropy at 5 kOe magnetic field. We have performed zero-field and longitudinal field Muon spin relaxation ($\mu$SR) studies on Dy$_{2}$Zr$_{2}$O$_{7}$. Our zero field studies reveal the absence of both long-range ordering and spin freezing down to 62 mK. The $\mu$SR relaxation rate exhibits a temperature-independent plateau below 4 K, indicating a dynamic ground state of fluctuating spins similar to the well-known spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$. The low-temperature spin fluctuations persist in the longitudinal field of 20 kOe as well and show unusual field dependence of the relaxation rate, which is uncommon for a spin-liquid system. Our results, combined with the previous studies do not show any evidence of spin ice or spin glass ground state, rather point to a disorder-induced dynamic magnetic ground state in the Dy$_{2}$Zr$_{2}$O$_{7}$ material.
Comment: 6 pages, 5 figures
Document Type: Working Paper
Access URL: http://arxiv.org/abs/2303.14426
Accession Number: edsarx.2303.14426
Database: arXiv
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