Chirality selective magnon-phonon hybridization and magnon-induced chiral phonons in a layered zigzag antiferromagnet

Bibliographic Details
Title: Chirality selective magnon-phonon hybridization and magnon-induced chiral phonons in a layered zigzag antiferromagnet
Authors: Cui, Jun, Bostroem, Emil Vinas, Ozerov, Mykhaylo, Wu, Fangliang, Jiang, Qianni, Chu, Jiun-Haw, Li, Changcun, Liu, Fucai, Xu, Xiaodong, Rubio, Angel, Zhang, Qi
Source: Nature Communications 14, 3396 (2023)
Publication Year: 2023
Collection: Condensed Matter
Subject Terms: Condensed Matter - Materials Science
More Details: Two-dimensional (2D) magnetic systems possess versatile magnetic order and can host tunable magnons carrying spin angular momenta. Recent advances show angular momentum can also be carried by lattice vibrations in the form of chiral phonons. However, the interplay between magnons and chiral phonons as well as the details of chiral phonon formation in a magnetic system are yet to be explored. Here, we report the observation of magnon-induced chiral phonons and chirality selective magnon-phonon hybridization in a layered zigzag antiferromagnet (AFM) FePSe$_3$. With a combination of magneto-infrared and magneto-Raman spectroscopy, we observe chiral magnon polarons (chiMP), the new hybridized quasiparticles, at zero magnetic field. The hybridization gap reaches 0.25~meV and survives down to the quadrilayer limit. Via first principle calculations, we uncover a coherent coupling between AFM magnons and chiral phonons with parallel angular momenta, which arises from the underlying phonon and space group symmetries. This coupling lifts the chiral phonon degeneracy and gives rise to an unusual Raman circular polarization of the chiMP branches. The observation of coherent chiral spin-lattice excitations at zero magnetic field paves the way for angular momentum-based hybrid phononic and magnonic devices.
Document Type: Working Paper
DOI: 10.1038/s41467-023-39123-y
Access URL: http://arxiv.org/abs/2302.10656
Accession Number: edsarx.2302.10656
Database: arXiv
More Details
DOI:10.1038/s41467-023-39123-y