Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$

Bibliographic Details
Title: Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$
Authors: Opletal, Petr, Sakai, Hironori, Haga, Yoshinori, Tokiwa, Yoshifumi, Yamamoto, Etsuji, Kambe, Shinsaku, Tokunaga, Yo
Publication Year: 2022
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science
More Details: We investigate the physical properties of a single crystal of uranium telluride U$_{7}$Te$_{12}$. We have confirmed that U$_{7}$Te$_{12}$ crystallizes in the hexagonal structure with three nonequivalent crystallographic uranium sites. The paramagnetic moments are estimated to be approximately 1 $\mu_{\rm B}$ per the uranium site, assuming a uniform moment on all the sites. A ferromagnetic phase transition occurs at $T_{\rm C}=48$ K, where the in-plane magnetization increases sharply, whereas the out-of-plane component does not increase significantly. With decreasing temperature further below $T_{\rm C}$ under field-cooling conditions, the out-of-plane component increases rapidly around $T^{\star}=26$ K. In contrast, the in-plane component hardly changes at $T^{\star}$. Specific heat measurement indicates no $\lambda$-type anomaly around $T^{\star}$, so this is a cross-over suggesting a reorientation of the ordering moments or successive magnetic ordering on the part of the multiple uranium sites.
Document Type: Working Paper
DOI: 10.7566/JPSJ.92.034704
Access URL: http://arxiv.org/abs/2211.16760
Accession Number: edsarx.2211.16760
Database: arXiv
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Items – Name: Title
  Label: Title
  Group: Ti
  Data: Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$
– Name: Author
  Label: Authors
  Group: Au
  Data: <searchLink fieldCode="AR" term="%22Opletal%2C+Petr%22">Opletal, Petr</searchLink><br /><searchLink fieldCode="AR" term="%22Sakai%2C+Hironori%22">Sakai, Hironori</searchLink><br /><searchLink fieldCode="AR" term="%22Haga%2C+Yoshinori%22">Haga, Yoshinori</searchLink><br /><searchLink fieldCode="AR" term="%22Tokiwa%2C+Yoshifumi%22">Tokiwa, Yoshifumi</searchLink><br /><searchLink fieldCode="AR" term="%22Yamamoto%2C+Etsuji%22">Yamamoto, Etsuji</searchLink><br /><searchLink fieldCode="AR" term="%22Kambe%2C+Shinsaku%22">Kambe, Shinsaku</searchLink><br /><searchLink fieldCode="AR" term="%22Tokunaga%2C+Yo%22">Tokunaga, Yo</searchLink>
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  Label: Publication Year
  Group: Date
  Data: 2022
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  Data: Condensed Matter
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  Data: <searchLink fieldCode="DE" term="%22Condensed+Matter+-+Strongly+Correlated+Electrons%22">Condensed Matter - Strongly Correlated Electrons</searchLink><br /><searchLink fieldCode="DE" term="%22Condensed+Matter+-+Materials+Science%22">Condensed Matter - Materials Science</searchLink>
– Name: Abstract
  Label: Description
  Group: Ab
  Data: We investigate the physical properties of a single crystal of uranium telluride U$_{7}$Te$_{12}$. We have confirmed that U$_{7}$Te$_{12}$ crystallizes in the hexagonal structure with three nonequivalent crystallographic uranium sites. The paramagnetic moments are estimated to be approximately 1 $\mu_{\rm B}$ per the uranium site, assuming a uniform moment on all the sites. A ferromagnetic phase transition occurs at $T_{\rm C}=48$ K, where the in-plane magnetization increases sharply, whereas the out-of-plane component does not increase significantly. With decreasing temperature further below $T_{\rm C}$ under field-cooling conditions, the out-of-plane component increases rapidly around $T^{\star}=26$ K. In contrast, the in-plane component hardly changes at $T^{\star}$. Specific heat measurement indicates no $\lambda$-type anomaly around $T^{\star}$, so this is a cross-over suggesting a reorientation of the ordering moments or successive magnetic ordering on the part of the multiple uranium sites.
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  Data: 10.7566/JPSJ.92.034704
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        Value: 10.7566/JPSJ.92.034704
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        Type: general
      – SubjectFull: Condensed Matter - Materials Science
        Type: general
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      – TitleFull: Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$
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            NameFull: Tokunaga, Yo
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