Electrically tunable moir\'e magnetism in twisted double bilayers of chromium triiodide

Bibliographic Details
Title: Electrically tunable moir\'e magnetism in twisted double bilayers of chromium triiodide
Authors: Cheng, Guanghui, Rahman, Mohammad Mushfiqur, Allcca, Andres Llacsahuanga, Rustagi, Avinash, Liu, Xingtao, Liu, Lina, Fu, Lei, Zhu, Yanglin, Mao, Zhiqiang, Watanabe, Kenji, Taniguchi, Takashi, Upadhyaya, Pramey, Chen, Yong P.
Source: Nat. Electron. 6 (2023) 434-442
Publication Year: 2022
Collection: Condensed Matter
Subject Terms: Condensed Matter - Materials Science
More Details: Moir\'e superlattices in van der Waals structures can be used to control the electronic properties of the material and lead to emergent correlated and topological phenomena. Its first demonstration in van der Waals magnets exhibited noncollinear states and domain structures with, however, limited manipulation. Here we report electrically tunable moir\'e magnetism in twisted double bilayers - that is, a bilayer plus a bilayer with a twist angle between them - of layered antiferromagnet CrI3. Using magneto-optical Kerr effect microscopy, we observe the coexistence of antiferromagnetic and ferromagnetic order with nonzero net magnetization - a hallmark of moir\'e magnetism. Such magnetic state extends over a wide range of twist angles (with transitions at around 0{\deg} and above 20{\deg}) and exhibits a nonmonotonic temperature dependence. We further demonstrate voltage-assisted magnetic switching. The observed nontrivial magnetic states and unprecedented control by twist angle, temperature and electrical gating are supported by the simulated phase diagram of the moir\'e magnetism.
Document Type: Working Paper
DOI: 10.1038/s41928-023-00978-0
Access URL: http://arxiv.org/abs/2204.03837
Accession Number: edsarx.2204.03837
Database: arXiv
More Details
DOI:10.1038/s41928-023-00978-0