Incommensurate-commensurate magnetic phase transition in the double tungstate Li2Co(WO4)2

Bibliographic Details
Title: Incommensurate-commensurate magnetic phase transition in the double tungstate Li2Co(WO4)2
Authors: Chen, Xiyu, Ding, Ning, Liu, Meifeng, Zou, Tao, Garlea, V. Ovidiu, Gong, Jingwen, Liu, Fei, Xie, Yunlong, Yang, Lun, Zheng, Shuhan, Wang, Xiuzhang, Dong, Shuai, Charlton, T., Liu, Jun-Ming
Publication Year: 2021
Collection: Condensed Matter
Subject Terms: Condensed Matter - Materials Science, Condensed Matter - Strongly Correlated Electrons
More Details: Magnetic susceptibility, specific heat, and neutron powder diffraction measurements have been performed on polycrystalline Li2Co(WO4)2 samples. Under zero magnetic field, two successive magnetic transitions at TN1 ~ 9.4 K and TN2 ~ 7.4 K are observed. The magnetic ordering temperatures gradually decrease as the magnetic field increases. Neutron diffraction reveals that Li2Co(WO4)2 enters an incommensurate magnetic state with a temperature dependent k between TN1 and TN2. The magnetic propagation vector locks-in to a commensurate value k = (1/2, 1/4, 1/4) below TN2. The antiferromagnetic structure is refined at 1.7 K with Co2+ magnetic moment 2.8(1) uB, consistent with our first-principles calculations.
Document Type: Working Paper
DOI: 10.1088/1674-1056/ac3818
Access URL: http://arxiv.org/abs/2111.04944
Accession Number: edsarx.2111.04944
Database: arXiv
More Details
DOI:10.1088/1674-1056/ac3818