Multiple Magnetic Bilayers and Unconventional Criticality without Frustration in BaCuSi$_2$O$_6$

Bibliographic Details
Title: Multiple Magnetic Bilayers and Unconventional Criticality without Frustration in BaCuSi$_2$O$_6$
Authors: Allenspach, S., Biffin, A., Stuhr, U., Tucker, G. S., Ohira-Kawamura, S., Kofu, M., Voneshen, D. J., Boehm, M., Normand, B., Laflorencie, N., Mila, F., Rüegg, Ch.
Source: Phys. Rev. Lett. 124, 177205 (2020)
Publication Year: 2019
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons
More Details: The dimerized quantum magnet BaCuSi$_2$O$_6$ was proposed as an example of "dimensional reduction" arising near the magnetic-field-induced quantum critical point (QCP) due to perfect geometrical frustration of its inter-bilayer interactions. We demonstrate by high-resolution neutron spectroscopy experiments that the effective intra-bilayer interactions are ferromagnetic, thereby excluding frustration. We explain the apparent dimensional reduction by establishing the presence of three magnetically inequivalent bilayers, with ratios 3:2:1, whose differing interaction parameters create an extra field-temperature scaling regime near the QCP with a non-trivial but non-universal exponent. We demonstrate by detailed quantum Monte Carlo simulations that the magnetic interaction parameters we deduce can account for all the measured properties of BaCuSi$_2$O$_6$, opening the way to a quantitative understanding of non-universal scaling in any modulated layered system.
Comment: 14 pages, 9 figures
Document Type: Working Paper
DOI: 10.1103/PhysRevLett.124.177205
Access URL: http://arxiv.org/abs/1911.04161
Accession Number: edsarx.1911.04161
Database: arXiv
More Details
DOI:10.1103/PhysRevLett.124.177205