Emergent units of itinerant spin-state excitations in LaCoO$_3$

Bibliographic Details
Title: Emergent units of itinerant spin-state excitations in LaCoO$_3$
Authors: Tomiyasu, K., Nomura, T., Kobayashi, Y., Ishihara, S., Ohira-Kawamura, S., Kofu, M.
Publication Year: 2018
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons
More Details: Spin crossover is expected to enrich unusual physical states in various types of condensed matter. Through inelastic neutron scattering, we study the spin-state excitations in the canonical and advanced platform, LaCoO$_3$, and reveal that the spatial correlation robustly maintains the seven-Co-site size below 300 K and the internal Co-$d$ electrons are spatially delocalized. By combining theoretical calculations, this dynamical short-range order is identified as a new collective unit for describing spin-state with dual spin-state nature beyond the conventional one-Co-site classification.
Comment: 11 pages, 7 figures, 1 table
Document Type: Working Paper
Access URL: http://arxiv.org/abs/1808.05888
Accession Number: edsarx.1808.05888
Database: arXiv
More Details
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