Magnetic structure of Ba(TiO)Cu$_4$(PO$_4$)$_4$ probed using spherical neutron polarimetry

Bibliographic Details
Title: Magnetic structure of Ba(TiO)Cu$_4$(PO$_4$)$_4$ probed using spherical neutron polarimetry
Authors: Babkevich, P., Testa, L., Kimura, K., Kimura, T., Tucker, G. S., Roessli, B., Rønnow, H. M.
Source: Phys. Rev. B 96, 214436 (2017)
Publication Year: 2017
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons
More Details: The antiferromagnetic compound Ba(TiO)Cu$_4$(PO$_4$)$_4$ contains square cupola of corner-sharing CuO$_4$ plaquettes, which were proposed to form effective quadrupolar order. To identify the magnetic structure, we have performed spherical neutron polarimetry measurements. Based on symmetry analysis and careful measurements we conclude that the orientation of the Cu$^{2+}$ spins form a non-collinear in-out structure with spins approximately perpendicular to the CuO$_4$ motif. Strong Dzyaloshinskii-Moriya interaction naturally lends itself to explain this phenomenon. The identification of the ground state magnetic structure should serve well for future theoretical and experimental studies into this and closely related compounds.
Comment: 9 pages, 4 figures
Document Type: Working Paper
DOI: 10.1103/PhysRevB.96.214436
Access URL: http://arxiv.org/abs/1709.08566
Accession Number: edsarx.1709.08566
Database: arXiv
More Details
DOI:10.1103/PhysRevB.96.214436