Surface-assisted carrier excitation in plasmonic nanostructure

Bibliographic Details
Title: Surface-assisted carrier excitation in plasmonic nanostructure
Authors: Shahbazyan, Tigran V.
Source: Plasmonics 13, 757 (2018)
Publication Year: 2017
Collection: Condensed Matter
Physics (Other)
Subject Terms: Condensed Matter - Mesoscale and Nanoscale Physics, Physics - Optics
More Details: We present a quantum-mechanical model for surface-assisted carrier excitation by optical fields in plasmonic nanostructures of arbitrary shape. We derive an explicit expression, in terms of local fields inside the metal structure, for surface absorbed power and surface scattering rate that determine the enhancement of carrier excitation efficiency near the metal-dielectric interface. We show that surface scattering is highly sensitive to the local field polarization, and can be incorporated into metal dielectric function along with phonon and impurity scattering. We also show that the obtained surface scattering rate describes surface-assisted plasmon decay (Landau damping) in nanostructures larger than the nonlocality scale. Our model can be used for calculations of plasmon-assisted hot carrier generation rates in photovoltaics and photochemistry applications.
Comment: 5 pages, 2 figures
Document Type: Working Paper
Access URL: http://arxiv.org/abs/1703.05874
Accession Number: edsarx.1703.05874
Database: arXiv
More Details
Description not available.