Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd$_{0.45}$Sr$_{0.55}$MnO$_3$ crystal

Bibliographic Details
Title: Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd$_{0.45}$Sr$_{0.55}$MnO$_3$ crystal
Authors: Izuchi, Y., Akaki, M., Akahoshi, D., Kuwahara, H.
Source: APL Materials 2, 022106 (2014)
Publication Year: 2014
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons
More Details: We have investigated the Mn-site substitution effect in Nd$_{0.45}$Sr$_{0.55}$MnO$_3$ single crystal, which has an $A$-type layered antiferromagnetic ($A$-AFM) phase with the 3$d_{x^2-y^2}$-type orbital-order. Substitution of Fe or Ga for Mn-site suppresses both the $A$-AFM order and competing ferromagnetic (FM) correlation whereas Cr substitution suppresses only the $A$-AFM order but reactivates the underlying FM correlation via double-exchange mechanism along the AFM coupled $c$-direction. In Nd$_{0.45}$Sr$_{0.55}$Mn$_{0.95}$Cr$_{0.05}$O$_3$, the $A$-AFM state with the orbital-order is changed into the orbital-disordered three-dimensional FM metallic state by applying magnetic field of $\mu_0 H = 12$ T, which is much smaller than that of the parent compound Nd$_{0.45}$Sr$_{0.55}$MnO$_3$.
Comment: 5 pages, 4 figures, to appear in APL Materials
Document Type: Working Paper
DOI: 10.1063/1.4866050
Access URL: http://arxiv.org/abs/1402.1543
Accession Number: edsarx.1402.1543
Database: arXiv
More Details
DOI:10.1063/1.4866050