Anomalous circular polarization of magneto-photoluminescence from individual CdSe nanocrystals

Bibliographic Details
Title: Anomalous circular polarization of magneto-photoluminescence from individual CdSe nanocrystals
Authors: Htoon, H., Crooker, S. A., Furis, M., Jeong, S., Efros, Al. L., Klimov, V. I.
Source: Physical Review Letters 102, 017402 (2009)
Publication Year: 2008
Collection: Condensed Matter
Subject Terms: Condensed Matter - Mesoscale and Nanoscale Physics, Condensed Matter - Materials Science
More Details: We study the low-temperature magneto-photoluminescence (PL) from individual CdSe nanocrystals. Nanocrystals having a small "bright" exciton fine structure splitting ($<$0.5 meV) exhibit a conventional left- and right-circularly polarized Zeeman PL doublet in applied magnetic fields. In contrast, nanocrystals with large fine structure splitting ($>$1 meV) show an anomalous magneto-PL polarization, wherein the lower-energy peak becomes circularly polarized with increasing field, while the higher-energy peak remains linearly polarized. This unusual behavior arises from strong mixing between the absorbing and emitting bright exciton levels due to strong anisotropic exchange interactions.
Comment: 15 pages, 3 figures; submitted
Document Type: Working Paper
DOI: 10.1103/PhysRevLett.102.017402
Access URL: http://arxiv.org/abs/0809.1116
Accession Number: edsarx.0809.1116
Database: arXiv
More Details
DOI:10.1103/PhysRevLett.102.017402