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Observation of Magnetic Field‐Induced and Partially Switchable Electric Polarization in Spin‐Chain FePbBiO4

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Title: Observation of Magnetic Field‐Induced and Partially Switchable Electric Polarization in Spin‐Chain FePbBiO4
Authors: Ajay Tiwari, D. Chandrasekhar Kakarla, Wei‐Lin Chen, C. Dhanasekhar, Ya‐Jing Hu, Jiunn‐Yuan Lin, Chin‐Wei Wang, Ting‐Wei Kuo, Arkadeb Pal, Mitch Ming‐Chi Chou, Hung‐Duen Yang
Source: Advanced Physics Research, Vol 3, Iss 11, Pp n/a-n/a (2024)
Publisher Information: Wiley-VCH, 2024.
Publication Year: 2024
Collection: LCC:Physics
Subject Terms: FePbBiO4, magnetic field‐induced, magnetoelectric effect, partially reversed electric polarization, Quasi‐one dimensional spin‐chain, switchable, Physics, QC1-999
More Details: Abstract The linear magnetoelectric (ME) characteristics of a quasi‐1D spin‐chain compound, FePbBiO4, are reported. Two distinct antiferromagnetic (AFM) orders occurring at ≈23 K (TN1) and 12 K (TN2) are verified using magnetization, specific heat, and conspicuous dielectric (ε′) anomalies. A striking observation is that no pyrocurrent (Ipy) is detected in the absence of magnetic field (H); however, H‐induced ferroelectric polarization (P) at TN1 and P unexpectedly partially switches or reverses below TN2 as reproduced by applying positive and negative electric fields (E). The resulting magnetic field and temperature (H‐T) phase diagram illustrates T‐dependent H‐induced spin reorientation and electric P. The interaction between T, H, spin dynamics, and lattice structures is pivotal and is qualitatively discussed and proposed as an explanation for the observed ME nature.
Document Type: article
File Description: electronic resource
Language: English
ISSN: 2751-1200
Relation: https://doaj.org/toc/2751-1200
DOI: 10.1002/apxr.202400056
Access URL: https://doaj.org/article/48215445be1941b687c97c2de0bf30d0
Accession Number: edsdoj.48215445be1941b687c97c2de0bf30d0
Database: Directory of Open Access Journals
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  Data: Observation of Magnetic Field‐Induced and Partially Switchable Electric Polarization in Spin‐Chain FePbBiO4
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  Data: <searchLink fieldCode="AR" term="%22Ajay+Tiwari%22">Ajay Tiwari</searchLink><br /><searchLink fieldCode="AR" term="%22D%2E+Chandrasekhar+Kakarla%22">D. Chandrasekhar Kakarla</searchLink><br /><searchLink fieldCode="AR" term="%22Wei‐Lin+Chen%22">Wei‐Lin Chen</searchLink><br /><searchLink fieldCode="AR" term="%22C%2E+Dhanasekhar%22">C. Dhanasekhar</searchLink><br /><searchLink fieldCode="AR" term="%22Ya‐Jing+Hu%22">Ya‐Jing Hu</searchLink><br /><searchLink fieldCode="AR" term="%22Jiunn‐Yuan+Lin%22">Jiunn‐Yuan Lin</searchLink><br /><searchLink fieldCode="AR" term="%22Chin‐Wei+Wang%22">Chin‐Wei Wang</searchLink><br /><searchLink fieldCode="AR" term="%22Ting‐Wei+Kuo%22">Ting‐Wei Kuo</searchLink><br /><searchLink fieldCode="AR" term="%22Arkadeb+Pal%22">Arkadeb Pal</searchLink><br /><searchLink fieldCode="AR" term="%22Mitch+Ming‐Chi+Chou%22">Mitch Ming‐Chi Chou</searchLink><br /><searchLink fieldCode="AR" term="%22Hung‐Duen+Yang%22">Hung‐Duen Yang</searchLink>
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  Data: Advanced Physics Research, Vol 3, Iss 11, Pp n/a-n/a (2024)
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  Data: Abstract The linear magnetoelectric (ME) characteristics of a quasi‐1D spin‐chain compound, FePbBiO4, are reported. Two distinct antiferromagnetic (AFM) orders occurring at ≈23 K (TN1) and 12 K (TN2) are verified using magnetization, specific heat, and conspicuous dielectric (ε′) anomalies. A striking observation is that no pyrocurrent (Ipy) is detected in the absence of magnetic field (H); however, H‐induced ferroelectric polarization (P) at TN1 and P unexpectedly partially switches or reverses below TN2 as reproduced by applying positive and negative electric fields (E). The resulting magnetic field and temperature (H‐T) phase diagram illustrates T‐dependent H‐induced spin reorientation and electric P. The interaction between T, H, spin dynamics, and lattice structures is pivotal and is qualitatively discussed and proposed as an explanation for the observed ME nature.
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        Value: 10.1002/apxr.202400056
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      – Text: English
    Subjects:
      – SubjectFull: FePbBiO4
        Type: general
      – SubjectFull: magnetic field‐induced
        Type: general
      – SubjectFull: magnetoelectric effect
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      – SubjectFull: partially reversed electric polarization
        Type: general
      – SubjectFull: Quasi‐one dimensional spin‐chain
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      – SubjectFull: switchable
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              Type: published
              Y: 2024
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