Hybridization gap in the heavy-fermion compound UPd$_2$Al$_3$ via quasiparticle scattering spectroscopy

Bibliographic Details
Title: Hybridization gap in the heavy-fermion compound UPd$_2$Al$_3$ via quasiparticle scattering spectroscopy
Authors: Jaggi, N. K., Mehio, O., Dwyer, M., Greene, L. H., Baumbach, R. E., Tobash, P. H., Bauer, E. D., Thompson, J. D., Park, W. K.
Source: Phys. Rev. B 95, 165123 (2017)
Publication Year: 2016
Collection: Condensed Matter
Subject Terms: Condensed Matter - Strongly Correlated Electrons
More Details: We present results from point-contact spectroscopy of the antiferromagnetic heavy-fermion superconductor UPd$_2$Al$_3$: conductance spectra are taken from single crystals with two major surface orientations as a function of temperature and magnetic field, and analyzed using a theory of co-tunneling into an Anderson lattice. Spectroscopic signatures are clearly identified including the distinct asymmetric double-peak structure arising from the opening of a hybridization gap when a coherent heavy Fermi liquid is formed. Both the hybridization gap, found to be 7.2 $\pm$ 0.3 meV at 4 K, and the conductance enhancement above a flat background decrease upon increasing temperature. While the hybridization gap is extrapolated to remain finite up to $\sim$28 K, close to the temperature around which the magnetic susceptibility displays a broad peak, the conductance enhancement vanishes at $\sim$18 K, slightly above the antiferromagnetic transition temperature ($T_\textrm{N}$ $\approx$ 14 K). This rapid decrease of the conductance enhancement is understood as a consequence of the junction drifting away from the ballistic regime due to increased scattering off magnons associated with the localized U 5$f$ electrons. This shows that while the hybridization gap opening is not directly associated with the antiferromagnetic ordering, its visibility in the conductance is greatly affected by the temperature-dependent magnetic excitations. Our findings are not only consistent with the 5$f$ dual-nature picture in the literature but also shed new light on the interplay between the itinerant and localized electrons in UPd$_2$Al$_3$.
Comment: 28 pages, 8 figures, published in Phys. Rev. B
Document Type: Working Paper
DOI: 10.1103/PhysRevB.95.165123
Access URL: http://arxiv.org/abs/1610.08601
Accession Number: edsarx.1610.08601
Database: arXiv
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  Data: Hybridization gap in the heavy-fermion compound UPd$_2$Al$_3$ via quasiparticle scattering spectroscopy
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  Data: <searchLink fieldCode="AR" term="%22Jaggi%2C+N%2E+K%2E%22">Jaggi, N. K.</searchLink><br /><searchLink fieldCode="AR" term="%22Mehio%2C+O%2E%22">Mehio, O.</searchLink><br /><searchLink fieldCode="AR" term="%22Dwyer%2C+M%2E%22">Dwyer, M.</searchLink><br /><searchLink fieldCode="AR" term="%22Greene%2C+L%2E+H%2E%22">Greene, L. H.</searchLink><br /><searchLink fieldCode="AR" term="%22Baumbach%2C+R%2E+E%2E%22">Baumbach, R. E.</searchLink><br /><searchLink fieldCode="AR" term="%22Tobash%2C+P%2E+H%2E%22">Tobash, P. H.</searchLink><br /><searchLink fieldCode="AR" term="%22Bauer%2C+E%2E+D%2E%22">Bauer, E. D.</searchLink><br /><searchLink fieldCode="AR" term="%22Thompson%2C+J%2E+D%2E%22">Thompson, J. D.</searchLink><br /><searchLink fieldCode="AR" term="%22Park%2C+W%2E+K%2E%22">Park, W. K.</searchLink>
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  Data: Phys. Rev. B 95, 165123 (2017)
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  Data: We present results from point-contact spectroscopy of the antiferromagnetic heavy-fermion superconductor UPd$_2$Al$_3$: conductance spectra are taken from single crystals with two major surface orientations as a function of temperature and magnetic field, and analyzed using a theory of co-tunneling into an Anderson lattice. Spectroscopic signatures are clearly identified including the distinct asymmetric double-peak structure arising from the opening of a hybridization gap when a coherent heavy Fermi liquid is formed. Both the hybridization gap, found to be 7.2 $\pm$ 0.3 meV at 4 K, and the conductance enhancement above a flat background decrease upon increasing temperature. While the hybridization gap is extrapolated to remain finite up to $\sim$28 K, close to the temperature around which the magnetic susceptibility displays a broad peak, the conductance enhancement vanishes at $\sim$18 K, slightly above the antiferromagnetic transition temperature ($T_\textrm{N}$ $\approx$ 14 K). This rapid decrease of the conductance enhancement is understood as a consequence of the junction drifting away from the ballistic regime due to increased scattering off magnons associated with the localized U 5$f$ electrons. This shows that while the hybridization gap opening is not directly associated with the antiferromagnetic ordering, its visibility in the conductance is greatly affected by the temperature-dependent magnetic excitations. Our findings are not only consistent with the 5$f$ dual-nature picture in the literature but also shed new light on the interplay between the itinerant and localized electrons in UPd$_2$Al$_3$.<br />Comment: 28 pages, 8 figures, published in Phys. Rev. B
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