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High quality MAPbBr3 films via pulsed laser deposition of single-crystalline targets.

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Title: High quality MAPbBr3 films via pulsed laser deposition of single-crystalline targets.
Authors: Ghavidel, E., Di Carlo, A., Ishteev, A., Barichello, J., Konstantinova, K., Saranin, D., Campanari, V., Martelli, F., Paci, B., Generosi, A., Guaragno, M., Cricenti, A., Becerrill, D., Luce, M., Matteocci, F., Di Trolio, A.
Source: Journal of Materials Chemistry C; 9/7/2024, Vol. 12 Issue 33, p13141-13148, 8p
Abstract: High quality MAPbBr3 films were grown by pulsed laser deposition of single-crystalline targets using an on-axis geometry. The gas ambience up to the mbar range and laser fluence of some tenths of Joule per square centimeter yielded single α-phase polycrystalline MAPbBr3 films, as revealed by ex situ XRD analysis. In situ low T studies allowed for the observation of cubic-to-tetragonal and of tetragonal-to-orthorombic phase transitions. Absorption and photoluminescence spectra show characteristic peaks around 2.35 eV. In particular, for thin films, PL measurements at low temperature showed narrow peaks characteristic of high crystalline quality and the absence of relevant defect-related recombination. The present results indicate a route to grow high quality thin films of metal halide perovskites via PLD of single-crystalline targets. [ABSTRACT FROM AUTHOR]
Copyright of Journal of Materials Chemistry C is the property of Royal Society of Chemistry and its content may not be copied or emailed to multiple sites or posted to a listserv without the copyright holder's express written permission. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
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  Data: High quality MAPbBr<subscript>3</subscript> films via pulsed laser deposition of single-crystalline targets.
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  Data: Journal of Materials Chemistry C; 9/7/2024, Vol. 12 Issue 33, p13141-13148, 8p
– Name: Abstract
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  Group: Ab
  Data: High quality MAPbBr<subscript>3</subscript> films were grown by pulsed laser deposition of single-crystalline targets using an on-axis geometry. The gas ambience up to the mbar range and laser fluence of some tenths of Joule per square centimeter yielded single α-phase polycrystalline MAPbBr<subscript>3</subscript> films, as revealed by ex situ XRD analysis. In situ low T studies allowed for the observation of cubic-to-tetragonal and of tetragonal-to-orthorombic phase transitions. Absorption and photoluminescence spectra show characteristic peaks around 2.35 eV. In particular, for thin films, PL measurements at low temperature showed narrow peaks characteristic of high crystalline quality and the absence of relevant defect-related recombination. The present results indicate a route to grow high quality thin films of metal halide perovskites via PLD of single-crystalline targets. [ABSTRACT FROM AUTHOR]
– Name: Abstract
  Label:
  Group: Ab
  Data: <i>Copyright of Journal of Materials Chemistry C is the property of Royal Society of Chemistry and its content may not be copied or emailed to multiple sites or posted to a listserv without the copyright holder's express written permission. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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              Text: 9/7/2024
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