Towards Informatics-Driven Design of Nuclear Waste Forms

Authors: Hegde, Vinay I., Peterson, Miroslava, Allec, Sarah I., Lu, Xiaonan, Mahadevan, Thiruvillamalai, Nguyen, Thanh, Kalahe, Jayani, Oshiro, Jared, Seffens, Robert J., Nickerson, Ethan K., Du, Jincheng, Riley, Brian J., Vienna, John D., Saal, James E.

Subject Terms: Condensed Matter - Materials Science

Access URL: http://arxiv.org/abs/2405.09897

Evaluation of GlassNet for physics-informed machine learning of glass stability and glass-forming ability

Authors: Allec, Sarah I., Lu, Xiaonan, Cassar, Daniel R., Nguyen, Xuan T., Hegde, Vinay I., Mahadevan, Thiruvillamalai, Peterson, Miroslava, Du, Jincheng, Riley, Brian J., Vienna, John D., Saal, James E.

Subject Terms: Condensed Matter - Materials Science, Computer Science - Machine Learning

Access URL: http://arxiv.org/abs/2403.10682

Glass and ceramic nuclear waste forms: The scientific battle.

Authors: Gregg, Daniel J. (AUTHOR), McCloy, John S. (AUTHOR), Vienna, John D. (AUTHOR), Macfarlane, Allison M. (AUTHOR), Weber, William J. (AUTHOR), Lumpkin, Gregory R. (AUTHOR)

Source: Bulletin of the Atomic Scientists. Jan2025, Vol. 81 Issue 1, p3-16. 14p.

Subjects: FUEL cycle, GLASS waste, WASTE treatment, INDUSTRIAL wastes, CERAMIC materials, RADIOACTIVE wastes, RADIOACTIVE waste disposal

Temperature and composition dependence modeling of viscosity and electrical conductivity of low-activity waste glass melts

Authors: Ferkl, Pavel, Lu, Xiaonan, Kruger, Albert A., Vienna, John D.

Source: In Journal of Non-Crystalline Solids 15 September 2024 640

Glass formulation and lab-scale testing of glasses designed for in-can Melter and in-container Vitrification of high-assay low-enriched uranium aqueous polishing Raffinate waste

Authors: Oshiro, Jared M., Gervasio, Vivianaluxa, Crum, Jarrod V., Riley, Brian J., Reiser, Joelle T., Snyder, Michelle M. Valenta, Dixon, Derek R., Nienhuis, Emily T., Droubay, Timothy C., Vienna, John D.

Source: In Journal of Nuclear Materials 15 August 2024 597

Insights on the structure and properties of sodium iron phosphate glasses from molecular dynamics simulations

Authors: Kalahe, Jayani, Mahadevan, T.S., Lu, Xiaonan, Vienna, John D., Riley, Brian J., Du, Jincheng

Source: In Journal of Nuclear Materials June 2024 594

Glass design using machine learning property models with prediction uncertainties: Nuclear waste glass formulation

Authors: Lu, Xiaonan, Weller, Zachary D., Gervasio, Vivianaluxa, Vienna, John D.

Source: In Journal of Non-Crystalline Solids 1 May 2024 631

Hanford low-activity waste vitrification: A review

Authors: Marcial, José, Riley, Brian J., Kruger, Albert A., Lonergan, Charmayne E., Vienna, John D.

Source: In Journal of Hazardous Materials 5 January 2024 461

Predicting initial dissolution rates using structural features from molecular dynamics simulations

Authors: Lu, Xiaonan, Deng, Lu, Gin, Stéphane, Parruzot, Benjamin, Reiser, Joelle T., Ryan, Joseph V., Vienna, John D., Du, Jincheng

Source: Journal of the American Ceramic Society. 106(2):1025-1036

Availability: http://explore.bl.uk/primo_library/libweb/action/display.do?tabs=detailsTab&gathStatTab=true&ct=display&fn=search&doc=ETOCvdc_100170280987.0x000001&indx=1&recIds=ETOCvdc_100170280987.0x000001

Formulation and testing of a high-tin borosilicate nuclear waste glass for in-can melting

Authors: Crum, Jarrod V., Vienna, John D., Riley, Brian J., Silverstein, Joshua A., Kissinger, Ryan M., Neeway, James J., George, Jaime L., Bellofatto, Diana L., Hall, Mark A.

Source: In Journal of Nuclear Materials November 2023 585

Durability evaluation of glasses to immobilize Fukushima (1F) secondary waste using ASTM C1220 (MCC-1) testing

Authors: Parruzot, Benjamin, Reiser, Joelle T., Lu, Xiaonan, Crum, Jarrod V., Reyes, Richard A., Finucane, Kevin G., Witwer, Keith S., Abeta, Sadaaki, Yoshioka, Masahiro, Vienna, John D.

Source: In Journal of Non-Crystalline Solids: X September 2023 19

Glass formulation and composition optimization with property models: A review.

Authors: Lu, Xiaonan¹ (AUTHOR) xiaonan.lu@pnnl.gov, Vienna, John D.¹ (AUTHOR), Du, Jincheng² (AUTHOR)

Source: Journal of the American Ceramic Society. Mar2024, Vol. 107 Issue 3, p1603-1624. 22p.

Subject Terms: *GLASS construction, *GLASS, *MACHINE learning, *GLASS structure

Fabrication of radioactive and non-radioactive titanate and zirconate ceramics for immobilization of used nuclear fuel

Authors: Reiser, Joelle T., Tolman, Kevin R., Kropp, Morgan T., Kissinger, Ryan M., Saslow, Sarah A., Cutforth, Derek A., Crum, Jarrod V., Seiner, Brienne N., Smith, Gary L., Vienna, John D.

Source: In Journal of Nuclear Materials 15 December 2022 572

Effects of Al:Si and (Al+Na):Si ratios on the static corrosion of sodium‐boroaluminosilicate glasses

Authors: Reiser, Joelle T., Parruzot, Benjamin, Gin, Stéphane, Bonnett, Jeffrey F., Smoljan, Courtney S., Seymour, Lorraine M., Ryan, Joseph V., Vienna, John D.

Source: International journal of applied glass science. 13(1):94-111

Availability: http://explore.bl.uk/primo_library/libweb/action/display.do?tabs=detailsTab&gathStatTab=true&ct=display&fn=search&doc=ETOCvdc_100136680802.0x000001&indx=1&recIds=ETOCvdc_100136680802.0x000001

Hanford low‐activity waste glass composition‐temperature‐melt viscosity relationships

Authors: Heredia‐Langner, Alejandro, Gervasio, Vivianaluxa, Cooley, Scott K., Lonergan, Charmayne E., Kim, Dong‐Sang, Kruger, Albert A., Vienna, John D.

Source: International journal of applied glass science. 13(4):514-525

Availability: http://explore.bl.uk/primo_library/libweb/action/display.do?tabs=detailsTab&gathStatTab=true&ct=display&fn=search&doc=ETOCvdc_100159567170.0x000001&indx=1&recIds=ETOCvdc_100159567170.0x000001

Heat capacity of complex aluminoborosilicate glasses

Authors: George, Jaime L., Sugawara, Toru, Ohira, Toshiaki, Kruger, Albert A., Vienna, John D.

Source: International journal of applied glass science. 13(4):576-590

Availability: http://explore.bl.uk/primo_library/libweb/action/display.do?tabs=detailsTab&gathStatTab=true&ct=display&fn=search&doc=ETOCvdc_100159567113.0x000001&indx=1&recIds=ETOCvdc_100159567113.0x000001

Redox chemistry of plutonium and plutonium surrogates in vitrified nuclear wastes

Authors: Darab, John G., Li, Hong, Bucher, Jerome J., Icenhower, Jonathan P., Allen, Patrick G., Shuh, David K., Vienna, John D.

Source: Journal of the American Ceramic Society. 105(11):6627-6639

Availability: http://explore.bl.uk/primo_library/libweb/action/display.do?tabs=detailsTab&gathStatTab=true&ct=display&fn=search&doc=ETOCvdc_100159568633.0x000001&indx=1&recIds=ETOCvdc_100159568633.0x000001

Impacts of temperature on sulfur solubility in low‐activity waste glasses

Authors: Jin, Tongan, Skidmore, Chloe H., Kruger, Albert A., Vienna, John D.

Source: International journal of applied glass science. 13(2):244-253

Availability: http://explore.bl.uk/primo_library/libweb/action/display.do?tabs=detailsTab&gathStatTab=true&ct=display&fn=search&doc=ETOCvdc_100151085198.0x000001&indx=1&recIds=ETOCvdc_100151085198.0x000001

Compositional dependence of crystallization and chemical durability in alkali aluminoborosilicate glasses

Authors: Deshkar, Ambar, Parruzot, Benjamin, Youngman, Randall E., Gulbiten, Ozgur, Vienna, John D., Goel, Ashutosh

Source: In Journal of Non-Crystalline Solids 15 August 2022 590

Structure–property relations of sodium iron phosphate nuclear waste glasses: Effects of iron redox ratio and glass composition.

Authors: Kalahe, Jayani¹, Lu, Xiaonan², Riley, Brian J.², Vienna, John D.², Du, Jincheng¹, du@unt.edu

Source: Journal of the American Ceramic Society; Feb2025, Vol. 108 Issue 2, p1-20, 20p